基于卫星遥感的大气污染物和温室气体排放反演

Satellite-based emission retrievals of air pollutants and greenhouse gases

  • 摘要: 基于卫星遥感的大气污染物和温室气体排放反演研究,为全面认识这些关键大气成分来源、精准实施减排措施提供了不可或缺的信息和数据基础。国内外相关研究在过去二十年中有了长足的发展,其中中国学者为领域发展做出了重要贡献,同时也对中国环境保护和碳中和事业提供了重要的科学支撑。在中国气象学会成立100周年之际,文中系统梳理中国学者近二十年来在星基排放反演方面的研究进展。首先,对常用排放反演方法进行简要总结,包括资料同化、局地质量平衡、高斯模型、二维模型、机器学习等。在此基础上,展示中国学者在氮氧化物(NOx)、氨气(NH3)、甲醛(HCHO)、乙二醛(CHOCHO)、二氧化硫(SO2)和一氧化碳(CO)等大气污染物,以及二氧化碳(CO2)和甲烷(CH4)等温室气体排放(和碳汇)反演的研究成果。最后,探讨反演方法和反演物种的历史演化进程、当前所面临的主要挑战和未来可能的发展方向,以期进一步推动大气污染物和温室气体排放的准确定量。

     

    Abstract: Satellite-based emission retrievals of atmospheric pollutants and greenhouse gases provide indispensable information and data foundation for comprehensive understanding of the sources of these key atmospheric compositions and precise implementation of emission reduction measures. Great advances have been made in the field of emission retrievals over the past two decades, and scientists in China have made substantial contributions to this field. Such studies have provided important scientific support for environmental protection and carbon neutrality in China. To celebrate the 100th anniversary of the Chinese Meteorological Society, this paper systematically reviews research progresses in China in satellite-based emission retrievals in the past two decades. Several widely used retrieval methods, including data assimilation, local mass balance, Gaussian models, two-dimensional models and machine learning, are briefly summarized.Studies on emission retrievals of atmospheric pollutants, including nitrogen oxides (NOx), ammonia (NH3), formaldehyde (HCHO), glyoxal (CHOCHO), sulfur dioxide (SO2) and carbon monoxide (CO), as well as greenhouse gases, including carbon dioxide (CO2) and methane (CH4) performed by Chinese scholars are presented. Finally, historical evolution of retrieval methods and target species as well as challenges in current satellite-based emission retrievals and future research directions are discussed to promote more accurate quantification of atmospheric pollutants and greenhouse gas emissions.

     

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